• Correlation between Wettability and Dissolution of Calcite in Ion-Free Water 

      AlMahri, Mariam; Lu, Jin-You; Chen, Shih-Wen; Olukan, Tuza Adeyemi; Yang, Thomas Chung-Kuang; Alhassan, Saeed; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2024-03-13)
      Calcite, a prevalent mineral in the earth’s crust, plays a pivotal role in various geological and industrial processes, including carbon sequestration, water treatment, and enhanced oil recovery. Understanding how wettability (a crucial surface property influenced by the interaction between calcite and surrounding fluids) affects calcite’s dissolution is essential for optimizing these processes. We ...
    • Direct growth of single-layer terminated vertical graphene array on germanium by plasma enhanced chemical vapor deposition 

      Al-Hagri, Abdulrahman; Li, Ru; Rajput, Nitul S; Lu, Jin-You; Cong, Shan; Sloyan, Karen; Almahri, Mariam Ali; Tamalampudi, Srinivasa Reddy; Chiesa, Matteo; Al Ghaferi, Amal (Journal article; Tidsskriftartikkel; Peer reviewed, 2019-08-26)
      Vertically aligned graphene nanosheet arrays (VAGNAs) exhibit large surface area, excellent electron transport properties, outstanding mechanical strength, high chemical stability, and enhanced electrochemical activity, which makes them highly promising for application in supercapacitors, batteries, fuel cell catalysts, etc. It is shown that VAGNAs terminated with a high-quality single-layer graphene ...
    • Direct Measurement of the Magnitude of the van der Waals Interaction of Single and Multilayer Graphene 

      Chiou, Yu-Cheng; Olukan, Tuza Adeyemi; Almahri, Mariam Ali; Apostoleris, Harry; Chiu, Cheng Hsiang; Lai, Chia-Yun; Lu, Jin-You; Santos, Sergio; Almansouri, Ibraheem; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2018-09-23)
      Vertical stacking of monolayers via van der Waals (vdW) assembly is an emerging field that opens promising routes toward engineering physical properties of two-dimensional materials. Industrial exploitation of these engineering heterostructures as robust functional materials still requires bounding their measured properties so as to enhance theoretical tractability and assist in experimental designs. ...
    • Discerning the Contribution of Morphology and Chemistry in Wettability Studies 

      Sloyan, Karen; Lai, Chia-Yun; Lu, Jin-You; Alfakes, Boulos; Al Hassan, Saeed; Almansouri, Ibraheem; Dahlem, Marcus S; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2018-07-15)
      The wetting behavior of homogeneous systems is now well understood at the macroscopic scale. However, this understanding offers little predictive power regarding wettability when mesoscopic chemical and morphological heterogeneities come into play. The fundamental interest in the effect of heterogeneity on wettability is derived from its high technological relevance in several industries, including ...
    • Enhanced photoelectrochemical performance of atomic layer deposited Hf-doped ZnO 

      Alfakes, Boulos; Garlisi, Corrado; Villegas, Juan; Al-Hagri, Abdulrahman; Tamalampudi, Srinivasa Reddy; Rajput, Nitul S.; Lu, Jin-You; Lewin, Erik; Sá, Jacinto; Almansouri, Ibraheem; Palmisano, Giovanni; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2020-01-08)
      Generation of hydrogen using photoelectrochemical (PEC) water splitting has attracted researchers for the last two decades. Several materials have been utilized as a photoanode in a water splitting cell, including ZnO due to its abundance, low production cost and suitable electronic structure. Most research attempts focused on doping ZnO to tailor its properties for a specific application. In this ...
    • The evolution in graphitic surface wettability with first-principles quantum simulations: the counterintuitive role of water 

      Lu, Jin-You; Lai, Chia-Yun; Almansoori, Ibraheem; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2018-08-08)
      The surface wettability of graphite has gained a lot of interest in nanotechnology and fundamental studies alike, but the types of adsorptions that dominate its time resolved surface property variations in ambient environment are still elusive. Prediction of the intrinsic surface wettability of graphite from first-principles simulations offers an opportunity to clarify the overall evolution. In this ...
    • Hybrid graphene metasurface for near-infrared absorbers 

      Mahfuzur Rahman, MD; Raza, Aikifa; Younes, Hammad; Alghaferi, Amal; Chiesa, Matteo; Lu, Jin-You (Journal article; Tidsskriftartikkel; Peer reviewed, 2019-08-19)
      We experimentally demonstrated an amorphous graphene-based metasurface yielding near-infrared super absorber characteristic. The structure is obtained by alternatively combining magnetron-sputtering deposition and graphene transfer coating fabrication techniques. The thickness constraint of the physical vapor–deposited amorphous metallic layer is unlocked and as a result, the as-fabricated graphene-based ...
    • Investigating the Ubiquitous Presence of Nanometric Water Films on Surfaces 

      Santos Hernandez, Sergio; Amadei, Carlo Alberto; Lai, Chia-Yun; Olukan, Tuza Adeyemi; Lu, Jin-You; Font, Josep; Barcons, Victor; Verdaguer, Albert; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2021-06-25)
      When we speak of nanometric water films on surfaces we are speaking about a truly ubiquitous phenomenon in nature. All surfaces exposed to ambient conditions are covered by a thin film of water that affects or mediates surface chemistry, general physical-chemical processes on surfaces, and even solid–solid interactions. We have investigated this phenomenon for over a decade by exploiting dynamic ...
    • Revealing the Quasi-Periodic Crystallographic Structure of Self-Assembled SnTiS3 Misfit Compound 

      Rajput, Nitul S.; Baik, Hionsuck; Lu, Jin-You; Tamalampudi, Srinivasa Reddy; Sankar, Raman; Al Ghaferi, Amal; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2021-04-28)
      Chemical vapor transport synthesis of SnTiS3 yields a self-assembled heterostructure of two distinct constituent materials, the semiconductor SnS and the semimetal TiS2. The misfit layer compound, although thermodynamically stable, is structurally complex, and precise understanding of the structure is necessary for designing nanoengineered heterojunction compound devices or for theoretical studies. ...
    • Superposition of semiconductor and semi-metal properties of self-assembled 2D SnTiS3 heterostructures 

      Tamalampudi, Srinivasa Reddy; Lu, Jin-You; Rajput, Nitul; Alfakes, Boulos; Sankar, Raman; Apostoleris, Harry; Patole, Shashikant; Almansouri, Ibraheem; Chiesa, Matteo (Journal article; Tidsskriftartikkel; Peer reviewed, 2020-07-15)
      Two-dimensional metal dichalcogenide/monochalcogenide thin flakes have attracted much attention owing to their remarkable electronic and electrochemical properties; however, chemical instability limits their applications. Chemical vapor transport (CVT)- synthesized SnTiS<sub>3</sub> thin flakes exhibit misfit heterojunction structure and are highly stable in ambient conditions, offering a ...
    • Thickness-Dependent Resonant Raman and E' Photoluminescence Spectra of Indium Selenide and Indium Selenide/Graphene Heterostructures 

      Tamalampudi, Srinivasa Reddy; Sankar, Raman; Apostoleris, Harry; Almahri, Mariam Ali; Alfakes, Boulos; Al-Hagri, Abdulrahman; Li, Ru; Gougam, Adel; Almansouri, Ibraheem; Chiesa, Matteo; Lu, Jin-You (Journal article; Tidsskriftartikkel; Peer reviewed, 2019-05-28)
      Atomically thin, two-dimensional (2D) indium selenide (InSe) has attracted considerable attention because of the dependence of its bandgap on sample thickness, making it suitable for small-scale optoelectronic device applications. In this work, by the use of Raman spectroscopy with three different laser wavelengths, including 488, 532, and 633 nm, representing resonant, near-resonant, and conventional ...